Screen printed flexible Bi₂Te₃-Sb₂Te₃based thermoelectric generator

This paper reports the fabrication and testing of Bismuth Tellurium (Bi2Te3) – Antimony Tellurium (Sb2Te3) based thermocouples using screen printing technology. In this study, screen printable thermoelectric pastes were developed and the transport properties of cured material were measured. The dimension of each planer thermoleg is 39.3 mm × 3 mm with a thickness of 67 µm for Bi2Te3 leg and 62 µm for Sb2Te3 leg. A single thermocouple with this dimension can generate a voltage of 6 mV and a peak output power of 48 nW at a temperature difference of 20°C. The calculated Seebeck coefficient of a single thermocouple is in the range of 262 to 282 µV/K. The Seebeck coefficient at room temperature were measured to be -134 to -119 µV/K and 128 to 134 µV/K for Bi2Te3 and Sb2Te3 respectively. This work demonstrates that the low-cost screen printing technology and low-temperature materials are promising for the fabrication of flexible thermoelectric generators (TEGs).