Self-induced generation of absolute negative temperatures in a multimode dense photon gas

Statistical mechanics connect macroscopic properties of matter with the laws governing the evolution of its microscopic constituents. In a classical gas, different thermodynamic laws apply to the weakly or strongly interacting particles of an ideal or real gas, respectively. Here, we demonstrate that a similar situation occurs for a gas of photons, which is contained in a multimode waveguide. We use a few-mode system provided by a standard step-index fiber operated below cutoff, which permits to prepare a high-density gas of photons. We show that, owing to the attractive potential energy contribution to the photon energy induced by the nonlinear Kerr effect, the mode population exhibits a spontaneous inversion from the fundamental to the highest order mode, as the input laser beam power grows larger. This inversion of the mode power distribution leads to a stable attractor for the output beam, and is associated with a progressive increase of the optical temperature until a flip of its sign leads to new regime of negative absolute temperatures. Our work demonstrates a new means to all-optically control the shape of laser beams.