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With the growing applications of maritime unmanned systems in environmental monitoring, ocean patrol, and emergency response, achieving efficient multi-platform cooperation in complex and dynamic marine environments remains a critical challenge. Unmanned Aerial Vehicles (UAVs) provide flexible and high-coverage sensing capabilities but are constrained by limited energy capacity, whereas Unmanned Surface Vehicles (USVs) offer long endurance and can serve as mobile platforms and energy supply nodes. Existing studies mostly focus on single-factor optimization, lacking a systematic analysis of the coupled relationships among energy, information (communication and positioning), and task decision making. To address this problem, this paper proposes an Energy–Information–Decision Coupling Optimization Method for Cooperative Maritime Unmanned Systems. A unified coupling model is established to integrate task completion, energy consumption, communication delay, and replenishment scheduling into a multi-objective optimization framework. A bi-level optimization algorithm is designed: the upper layer optimizes USV trajectories and energy supply strategies, while the lower layer optimizes UAV path planning and task allocation. A closed-loop adaptive mechanism is incorporated to achieve optimal cooperation under dynamic tasks and energy constraints. Extensive simulations combined with real-world experimental data are conducted to evaluate the method in terms of mission efficiency, energy balance, communication latency, and system robustness, with ablation studies quantifying the contribution of the coupling module. Results demonstrate that the proposed method significantly outperforms non-coupled or single-factor optimization strategies across multiple performance metrics: it achieves a task completion rate exceeding 93%, reduces total energy consumption by approximately 6% and replenishes waiting latency by over 28% compared with the decoupled baseline method. This effectively enhances the cooperative efficiency and robustness of maritime unmanned systems, and provides theoretical and methodological guidance for large-scale, complex ocean missions.