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Arch-suspended structures represent a distinctive form of hybrid suspension system. By combining an arch with a suspended floor system, this structural typology leverages the inherent advantages of both components while mitigating the limitations of each when used independently. This synergy effectively reduces peak internal forces and flexural deformations in structural members. Although widely applied in bridge engineering, research on arch-suspended building structures remains scarce. This paper investigates the construction techniques employed for a large-scale arch-suspended building. The stability of temporary support systems during construction is verified, and the mechanical behavior of critical joints—including the composite slab hanging pillar, arch support, and arch roof—is examined through both experimental testing and numerical simulation. The results demonstrate that a partitioned and segmented construction method is feasible for such complex structures. Structural internal forces and deformations can be effectively controlled by installing tubular temporary supports on both sides of the hanging pillars and lattice temporary supports at the base. Step-by-step unloading of these temporary supports ensures their stability throughout the construction process. Furthermore, the welds in the composite slab hanging pillar effectively transfer tensile forces from the middle plate to the side plates, enabling composite action and collaborative load-bearing among the steel plates. When subjected to loads of 2 times and 4.3 times the design load, localized plasticity was observed in the arch support and arch roof, respectively, while the overall structural integrity remained secure. This study provides a valuable reference for the design and construction of innovative long-span building structures, offering insights that can inform the development and practical application of arch-suspended systems in future architectural projects.