Search for a command to run...
<strong class="journal-contentHeaderColor">Abstract.</strong> Methane (CH<sub>4</sub>) and hydrogen (H<sub>2</sub>) play critical roles in atmospheric chemistry and climate processes. CH<sub>4</sub> is a powerful greenhouse gas, whereas H<sub>2</sub>, although not a greenhouse gas itself, indirectly affects radiative forcing by modifying the atmosphere's oxidative capacity and therefore the concentrations of CH<sub>4</sub>, ozone (O<sub>3</sub>) and stratospheric water vapor. Hydrogen is predominantly removed through microbial uptake in soils, while approximately 6 % of CH<sub>4</sub> is taken up by soils, a factor that contributes significantly to its overall atmospheric budget. Soil uptake depends on various soil characteristics, including type, temperature, moisture, and for CH<sub>4</sub>, nitrogen deposition. Accurately representing these influences requires a detailed understanding of both atmospheric conditions and land surface and hydrological properties. However, many Earth system models currently use fixed soil deposition rates for H<sub>2</sub> and CH<sub>4</sub>, without accounting for variations in soil properties. We present BIODEP, a new biogenic deposition submodel that has been integrated into the ECHAM/MESSy Atmospheric Chemistry model (EMAC). BIODEP dynamically simulates the uptake of CH<sub>4</sub> and H<sub>2</sub> by soil, based on local meteorological and soil conditions. With BIODEP, the soil sinks of CH<sub>4</sub> and H<sub>2</sub> are updated online based on the meteorological conditions, atmospheric composition, and land surface properties provided by the EMAC model. The EMAC model is coupled to the JSBACH land surface and vegetation model. This allows for a consistent and interactive treatment of soil sinks within the atmospheric chemistry model. Modeled global mean soil uptakes of 62.7 ± 11.7 Tg yr<sup>−1</sup> for H<sub>2</sub> and 30.2 ± 4.8 Tg yr<sup>−1</sup> for CH<sub>4</sub> are consistent with previous studies, and the resulting atmospheric mixing ratios show good agreement with observations from the NOAA GML Carbon Cycle Cooperative Global Air Sampling Network, evaluated over the period 2009–2019. In addition, comparison with column-averaged CH<sub>4</sub> (XCH<sub>4</sub>) observations from the Greenhouse Gases Observing Satellite (GOSAT) demonstrates that EMAC reproduces the global and zonal-scale methane distribution with small mean biases, providing independent support for the accuracy of the simulated soil methane sink. This development makes EMAC a state-of-the-art model to interactively simulate atmospheric chemistry, including both the soil sinks of CH<sub>4</sub> and H<sub>2</sub>. This enables more consistent simulation of trace gas budgets and an improved assessment of the feedbacks between land surface processes, atmospheric composition, and future climate and emission scenarios.